Thermo-osmotic ionogel enabled high-efficiency harvesting of low-grade heat

Wei Li, Yuchen Liu, Zimeng Zhang, Ruochen Liu, Jingjing Qiu, Shiren Wang

Research output: Contribution to journalArticlepeer-review

Abstract

Low efficiency in recovering low-grade heat remains unresolved despite decades of attempts. In this research, we designed and fabricated a novel thermo-osmotic ionogel (TOI) composite to recover low-grade heat to generate electric power through a thermo-induced ion gradient and selective ion diffusion. The TOI composite was assembled with a crystalline ionogel (polymer-confined LiNO3-3H2O) film, ion selective membrane, and hydrogel film. With a 90 °C heat supply, the single TOI composite produced a high open-circuit voltage of 0.52 V, a differential thermal voltage of ∼26 mV K−1, a peak power density of 0.4 W m−2, and a ground-breaking peak energy conversion efficiency of 11.17%. Eight pieces of such a TOI composite were connected in series, demonstrating an open-circuit voltage of 3.25 volts. Such a TOI system was also demonstrated to harvest body temperature for powering a LED, opening numerous opportunities in powering wearable devices.

Original languageEnglish
Pages (from-to)15755-15765
Number of pages11
JournalJournal of Materials Chemistry A
Volume9
Issue number28
DOIs
StatePublished - Jul 28 2021

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